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Acceleration of the particulate organic matter hydrolysis by start-up stage recovery and its original

Yanqing Duan, Aijuan Zhou, Xiuping Yue, Zhichun Zhang, Yanjuan Gao, Yanhong Luo, Xiao Zhang

《环境科学与工程前沿（英文）》 2021年 第15卷 第1期 doi: 10.1007/s11783-020-1304-3

摘要： Abstract • Carbon availability was partially solved by POM recovery and fermentation. • 12% carbon sources were regenerated by fermentation of the entrapped 35% TCOD. • The unique microbial communities facilitated the efficient hydrolysis of the POM. • Considerable economic benefits in aeration power and ECS dosage were anticipated. To address the availability of carbon sources for denitrification, the accelerated hydrolysis of the most abundant but low-availability fraction of particulate organic matter (POM) was investigated. Mesh sieves with different pore sizes were used as primary pretreatment at the start-up-stage of the biological process to separate some POM from the liquid system. The changes in soluble carbohydrates and proteins were monitored to investigate the hydrolysis performance of the sieved POM, with waste activated sludge (WAS) as the control test. The results showed that an average of 35% POM could be entrapped before filtrate mat development. In addition, benefiting from the high polysaccharides concentration, as well as the high availability due to the relatively loose physical structure, a 23% hydrolysis efficiency of POM was obtained, in contrast to that of WAS (3.4%), with a hydrolysis constant of 0.39 h−1. The prominent performance was also attributed to the unique microbial communities having been domesticated at a lower temperature, especially the cellulose-degrading bacteria Paraclostridium and psychrophile Psychrobacter, making up 6.94% and 2.56%, respectively. Furthermore, the potential benefits and application of improved POM hydrolysis by start-up stage recovery via mesh sieves combined with anaerobic fermentation were evaluated, including selective POM entrapment, alleviation of blockage and wear, and a reduction in aeration energy. By the proposed strategy, carbon availability for biological nutrient removal (BNR) processes is anticipated to be improved more economically than that can be achieved by primary clarifier elimination.

关键词： Particulate organic matter (POM)     Hydrolysis     Microbial community     Mass balance    

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Chemical characteristics of fine particulate matter emitted from commercial cooking

Bing PEI,Hongyang CUI,Huan LIU,Naiqiang YAN

《环境科学与工程前沿（英文）》 2016年 第10卷 第3期   页码 559-568 doi: 10.1007/s11783-016-0829-y

摘要： The chemical characteristics of fine particulate matter (PM ) emitted from commercial cooking were explored in this study. Three typical commercial restaurants in Shanghai, i.e., a Shanghai-style one (SHS), a Sichuan-style one (SCS) and an Italian-style one (ITS), were selected to conduct PM sampling. Particulate organic matter (POM) was found to be the predominant contributor to cooking-related PM mass in all the tested restaurants, with a proportion of 69.1% to 77.1%. Specifically, 80 trace organic compounds were identified and quantified by gas chromatography/mass spectrometry (GC/MS), which accounted for 3.8%–6.5% of the total PM mass. Among the quantified organic compounds, unsaturated fatty acids had the highest concentration, followed by saturated fatty acids. Comparatively, the impacts of other kinds of organic compounds were much smaller. Oleic acid was the most abundant single species in both SCS and ITS. However, in the case of SHS, linoleic acid was the richest one. ITS produced a much larger mass fraction of most organic species in POM than the two Chinese cooking styles except for monosaccharide anhydrides and sterols. The results of this study could be utilized to explore the contribution of cooking emissions to PM pollution and to develop the emission inventory of PM from cooking, which could then help the policy-makers design efficient treatment measures and control strategies on cooking emissions in the future.

关键词： commercial cooking     PM2.5     chemical characteristics     organic matter    

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Particulate matter 2.5 triggers airway inflammation and bronchial hyperresponsiveness in mice by activating

《医学前沿（英文）》 2021年 第15卷 第5期   页码 750-766 doi: 10.1007/s11684-021-0839-4

摘要： Exposure to particulate matter 2.5 (PM2.5) potentially triggers airway inflammation by activating nuclear factor-κB (NF-κB). Sirtuin 2 (SIRT2) is a key modulator in inflammation. However, the function and specific mechanisms of SIRT2 in PM2.5-induced airway inflammation are largely understudied. Therefore, this work investigated the mechanisms of SIRT2 in regulating the phosphorylation and acetylation of p65 influenced by PM2.5-induced airway inflammation and bronchial hyperresponsiveness. Results revealed that PM2.5 exposure lowered the expression and activity of SIRT2 in bronchial tissues. Subsequently, SIRT2 impairment promoted the phosphorylation and acetylation of p65 and activated the NF-κB signaling pathway. The activation of p65 triggered airway inflammation, increment of mucus secretion by goblet cells, and acceleration of tracheal stenosis. Meanwhile, p65 phosphorylation and acetylation, airway inflammation, and bronchial hyperresponsiveness were deteriorated in SIRT2 knockout mice exposed to PM2.5. Triptolide (a specific p65 inhibitor) reversed p65 activation and ameliorated PM2.5-induced airway inflammation and bronchial hyperresponsiveness. Our findings provide novel insights into the molecular mechanisms underlying the toxicity of PM2.5 exposure. Triptolide inhibition of p65 phosphorylation and acetylation could be an effective therapeutic approach in averting PM2.5-induced airway inflammation and bronchial hyperresponsiveness.

关键词： particulate matter 2.5     sirtuin 2     p65     airway inflammation     bronchial hyperresponsiveness     triptolide    

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Seasonal variations in leaf capturing of particulate matter, surface wettability and micromorphology

Huixia WANG, Hui SHI, Yangyang LI, Ya YU, Jun ZHANG

《环境科学与工程前沿（英文）》 2013年 第7卷 第4期   页码 579-588 doi: 10.1007/s11783-013-0524-1

摘要： The seasonal changes in leaf particulate matter (PM) accumulation, surface wettability and micromorphology in urban tree species, including ( . ), ( . ) and ( . ), were studied during a single growing season. The three species showed distinct seasonal trends in PM accumulation, increasing from spring to autumn (or winter) even during the rainy season, but at different rates. During the study, the leaf PM retention amount of , a species with ridged leaf surfaces, was significantly higher than that of and , species with waxy leaf surfaces. The contact angles of water droplets on leaves decreased with leaf age except on the abaxial surface of , which remained non-wettable or highly non-wettable throughout the growing season; the decrease in the contact angle on adaxial surface of was greater when compared with and . A significant and negative relationship existed between leaf PM retention amounts and contact angles on adaxial surface of leaves of all three species. The increase in wettability, probably caused when epicuticular wax was destroyed by mechanical and chemical abrasion, seemed to be the main factor leading to seasonal variations in leaf PM accumulation.

关键词： contact angle     particulate matter     retention amount    

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Particulate matter and metals partitioning in highway rainfall-runoff

Gaoxiang YING, John J. SANSALONE,

《环境科学与工程前沿（英文）》 2010年 第4卷 第1期   页码 35-46 doi: 10.1007/s11783-010-0009-4

摘要： This study investigated the particulate matter (PM) and metals in highway dry deposition and rainfall-runoff as a function of hydrologic transport and settling on an event basis. Events were differentiated as mass-limited (ML) and flow-limited (FL). Results indicate that unique and separate suspended sediment concentration (SSC) relationships with turbidity occurred for ML and FL events. Sixty minutes of quiescent settling produced a single SSC-turbidity relationship for all events. ML events transport higher proportions of settleable and sediment PM while FL events transported relatively higher suspended PM. For batch clarification with one hour of settling, ML events had generally higher treatment efficiencies compared to FL events for the same settling conditions. Highway dry deposition PM was hetero-disperse and coarse ( = 304 µm). Results indicate that the acidic rainfall is not a significant contributor to metals in runoff but is capable of leaching metals from dry deposition PM into runoff. Partitioning in retained runoff resulted in a particulate-bound €predominance €for €most €metals €except Ca and Mg. While the finer fraction of dry deposition PM (<75µm) generates the highest metal concentrations, the highest metal mass is associated with the coarser fraction (>75µm).

关键词： stormwater     particulate matter (PM)     turbidity     suspended sediment concentration (SSC)     unit operations     metals     dry deposition     acid rain    

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A method for quantifying bias in modeled concentrations and source impacts for secondary particulatematter

Cesunica E. Ivey, Heather A. Holmes, Yongtao Hu, James A. Mulholland, Armistead G. Russell

《环境科学与工程前沿（英文）》 2016年 第10卷 第5期 doi: 10.1007/s11783-016-0866-6

摘要： A method for quantifying source impacts for secondary PM species is derived. The method provides estimates of bias in modeled concentrations. Adjusted concentrations match corresponding observations at monitored locations. Sources impacts on secondary species are estimated over the US for 20 sources. Community Multi-Scale Air Quality (CMAQ) estimates of sulfates, nitrates, ammonium, and organic carbon are highly influenced by uncertainties in modeled secondary formation processes, such as chemical mechanisms, volatilization, and condensation rates. These compounds constitute the majority of PM mass, and reducing bias in estimated concentrations has benefits for policy measures and epidemiological studies. In this work, a method for adjusting source impacts on secondary species is developed that provides estimates of source contributions and reduces bias in modeled concentrations compared to observations. The bias correction adjusts concentrations and source impacts based on the difference between modeled concentrations and observations while taking into account uncertainties at the location of interest; and it is applied both spatially and temporally. We apply the method over the US for 2006. The mean bias for initial CMAQ concentrations compared to observations is −0.28 (OC), 0.11 (NO ), 0.05 (NH ), and −0.08 (SO ). The normalized mean bias in modeled concentrations compared to observations was effectively zero for OC, NO , NH , and SO after applying the secondary bias correction. 10-fold cross-validation was conducted to determine the performance of the spatial application of the bias correction. Cross-validation performance was favorable; correlation coefficients were greater than 0.69 for all species when comparing observations and concentrations based on kriged correction factors. The methods presented here address model uncertainties by improving simulated concentrations and source impacts of secondary particulate matter through data assimilation. Secondary-adjusted concentrations and source impacts from 20 emissions sources are generated for 2006 over continental US.

关键词： Particulate matter     Source apportionment     Secondary particulate matter     Chemical transport modeling     Receptor modeling    

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Concentrations of toxic heavy metals in ambient particulate matter in an industrial area of northeastern

PIAO Fengyuan, SUN Xiance, LIU Shuang, YAMAUCHI Toru

《医学前沿（英文）》 2008年 第2卷 第2期   页码 207-210 doi: 10.1007/s11684-008-0040-z

摘要： This paper investigates concentrations of various heavy metals in ambient particulate matter (PM) and provide evidence for prevention from air pollution. The concentrations of heavy metal components in the PM were determined by inductively coupled plasma/Mass spectrometry (ICP/MS) from September 2000 to August 2002 in a northeast industrial city in China. Concentrations of Cd, Mn, Pb, Ni, Cr and As in the PM were 9.3, 461.9, 588.7, 69.5, 205.7 and 57.4 ng/m in the industrial area, and 5.7, 245.5, 305.0, 31.4, 58.8 and 32.5 ng/m in the main road, respectively. Concentrations of these heavy metals except Cd were significantly higher in the industrial area and main road than those in the suburban area ( < 0.05 or < 0.01). The change curves of the six heavy metal concentrations show their concentrations increased in the winter and spring, but decreased in the summer and autumn. The results indicate that concentrations of the metals in the PM are relatively high in the industrial area and main road.

关键词： summer     August     northeast industrial     September     spring    

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Long-term trends of fine particulate matter and chemical composition in the Pearl River Delta Economic

Xuemei WANG,Weihua CHEN,Duohong CHEN,Zhiyong WU,Qi Fan

《环境科学与工程前沿（英文）》 2016年 第10卷 第1期   页码 53-62 doi: 10.1007/s11783-014-0728-z

摘要： Understanding the trends in PM levels is essential for formulating clean air plans. This paper analyzes PM data from various published sources for the years 2000 to 2010 in the Pearl River Delta Economic Zone (PRDEZ). The long-term variation in PM mass concentration is analyzed. Results show that PM , organic carbon (OC), elemental carbon (EC), and show a similar trend, increasing before 2005 and then decreasing slightly. The annual average PM concentration ranges from 49.1 μg·m in 2000 to 64.3 μg·m in 2010, with a peak of 84.1 μg·m in 2004. None of these 11 years meets the new National Ambient Air Quality standard (NAAQS) for PM (35 μg·m ). Overall average concentrations of OC, EC, and are 13.0, 6.5, and 11.8 μg·m , respectively. and respectively have concentrations of 1.5 μg·m and 2.9 μg·m in 2000 and 6.4 μg·m and 5.3 μg·m in 2010, with a statistically significant average annual trend of+ 0.2 μg·m ·yr and+ 0.1 μg·m ·yr . In certain geographic regions, OC and EC contribute most of the PM , while in other regions secondary water-soluble ions are more important. In general, OC and are the dominant components of PM , contributing 20.6% and 18.6%, respectively. These results provide, for the first time, a better understanding of the long-term PM characteristics and trends, on a species-by-species basis, in the PRDEZ. The results indicate that PM abatement needs to prioritize secondary species.

关键词： long-term trends     fine particulate matter     chemical components     Pearl River Delta Economic Zone (PRDEZ)    

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Photoaging mechanism of microplastics: a perspective on the effect of dissolved organic matter in natural

《环境科学与工程前沿（英文）》 2023年 第17卷 第11期 doi: 10.1007/s11783-023-1743-8

摘要：

● Microplastics (MPs) undergo photoaging in natural water under light irradiation.

关键词： Microplastics     Photoaging     Dissolved organic matter     ROS generation    

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Airborne bacteria associated with particulate matter from a highly urbanised metropolis: A potential

《环境科学与工程前沿（英文）》 2022年 第16卷 第9期 doi: 10.1007/s11783-022-1552-5

摘要：

• The airborne bacteria of Mexico City are representative of urban environments.

关键词： Airborne bacteria     Urbanisation     PM10     Mexico City     Microbiome    

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Determination of polyfluoroalkyl compounds in water and suspended particulate matter in the river Elbe

Lutz AHRENS, Merle PLASSMANN, Zhiyong XIE, Ralf EBINGHAUS

《环境科学与工程前沿（英文）》 2009年 第3卷 第2期   页码 152-170 doi: 10.1007/s11783-009-0021-8

摘要： The distribution of polyfluoroalkyl compounds (PFCs) in the dissolved and particulate phase and their discharge from the river Elbe into the North Sea were studied. The PFCs quantified included C -C perfluorinated sulfonates (PFSAs), 6∶2 fluorotelomer sulfonate (6∶2 FTS), C and C perfluorinated sulfinates (PFSiAs), C -C perfluorinated carboxylic acids (PFCAs), perfluoro-3,7-dimethyl-octanoic acid (3,7m -PFOA), perfluorooctane sulfonamide (FOSA), and n-ethyl perfluroctane sulfonamidoethanol (EtFOSE). PFCs were mostly distributed in the dissolved phase, where perfluorooctanoic acid (PFOA) dominated with 2.9-12.5 ng/L. In the suspended particulate matter FOSA and perfluorooctane sulfonate (PFOS) showed the highest concentrations (4.0 ng/L and 2.3 ng/L, respectively). The total flux of ∑PFCs from the river Elbe was estimated to be 802 kg/year for the dissolved phase and 152 kg/year for the particulate phase. This indicates that the river Elbe acts as a source of PFCs into the North Sea. However, the concentrations of perfluorobutane sulfonate (PFBS) and perfluorobutanoic acid (PFBA) in the North Sea were higher than that in the river Elbe, thus an alternative source must exist for these compounds.

关键词： polyfluoroalkyl compounds (PFCs)     perfluorooctane sulfonate (PFOS)     perfluorooctanoic acid (PFOA)     surface water     water-particulate partitioning    

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Identification of sources, characteristics and photochemical transformations of dissolved organic matter

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1340-z

摘要：

• The source of DOM in surface water and sediment is inconsistent.

关键词： Dissolved organic matter     Parallel factor analysis     Excitation-emission matrices     Photodegradation    

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Photosensitivity sources of dissolved organic matter from wastewater treatment plants and their mediation

《环境科学与工程前沿（英文）》 2023年 第17卷 第6期 doi: 10.1007/s11783-023-1669-1

摘要：

● EE2 photodegradation behavior in the presence of four WWTPs’ DOM was explored.

关键词： Photosensitivity sources     17α-ethinylestradiol     Photodegradation     Dissolved organic matter     Wastewater treatment plants    

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Assessing the premature death due to ambient particulate matter in China’s urban areas from 2004 to 2013

Guoxia MA, Jinnan WANG, Fang YU, Xiaomin GUO, Yanshen ZHANG, Chao LI

《环境科学与工程前沿（英文）》 2016年 第10卷 第5期 doi: 10.1007/s11783-016-0849-7

摘要： The number of annual premature deaths attributable to China’s air pollution ranged from 350000 to 520000 from 2004 to 2013, while the figure in 2013 reached 9.9% of total deaths in China. In 2004, the life expectancy potential years of life lost was 69.6 and 1.85 years respectively in contrast to 74.4 and 0.67 years respectively in 2013. The number of PYLL attributable to air pollution in the northern regions is found to be larger than that of the southern regions. The Environmental Burden of Disease (EBD) approach for outdoor air pollution has been used to calculate premature deaths and average potential years of life lost attributable to air pollution in China over the past 10 years with differences between the North and the South of the country being analyzed. The results indicate that: (1) Between 2004 and 2013, annual premature deaths attributable to outdoor air pollution in China ranged from 350000 to 520000. In 2013, deaths resulting from air pollution in China represented 9.9% of the country’s total deaths. (2) In 2004, the average life expectancy of the Chinese population and the number of potential years of life lost (PYLL) attributable to air pollution was 69.6 and 1.85 years respectively as compared to 74.4 and 0.67 years respectively in 2013. (3) The number of the PYLL attributable to air pollution in the northern regions of China is found to be larger than that of the southern regions. The PYLL figures of the northern and southern regions in 2004 were 2.3 and 1.8 years, respectively, with a difference of 0.5 years, as compared to 1.4 and 0.7 years respectively with a difference of 0.7 years in 2013.

关键词： Air pollution     Public health     Premature deaths     Health assessment    

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Dilution sampling and analysis of particulate matter in biomass-derived syngas

Xiaoliang WANG, Curtis ROBBINS, S. Kent HOEKMAN, Judith C. CHOW, John G. WATSON, Dennis SCHUETZLE

《环境科学与工程前沿（英文）》 2011年 第5卷 第3期   页码 320-330 doi: 10.1007/s11783-011-0347-x

摘要： Thermochemical biomass gasification, followed by conversion of the produced syngas to fuels and electrical power, is a promising energy alternative. Real-world characterization of particulate matter (PM) and other contaminants in the syngas is important to minimize damage and ensure efficient operation of the engines it powers and the fuels created from it. A dilution sampling system is demonstrated to quantify PM in syngas generated from two gasification plants utilizing different biomass feedstocks: a BioMax 15 Biopower System that uses raw and torrefied woodchips as feedstocks, and an integrated biorefinery (IBR) that uses rice hulls and woodchips as feedstocks. PM mass concentrations in syngas from the IBR downstream of the purification system were 12.8–13.7 μg·m , which were significantly lower than the maximum level for catalyst protection (500 μg·m ) and were 2–3 orders of magnitude lower than those in BioMax 15 syngas (2247–4835 μg·m ). Ultrafine particle number concentration and PM chemical constituents were also much lower in the IBR syngas than in the BioMax 15. The dilution sampling system enabled reliable measurements over a wide range of concentrations: the use of high sensitivity instruments allowed measurement at very low concentrations (~1 μg·m ), while the flexibility of dilution minimized sampling problems that are commonly encountered due to high levels of tars in raw syngas (~1 g·m ).

关键词： dilution source sampling     syngas characterization     biomass gasification     ultrafine particles    

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标题 作者 时间 类型 操作

Acceleration of the particulate organic matter hydrolysis by start-up stage recovery and its original

Yanqing Duan, Aijuan Zhou, Xiuping Yue, Zhichun Zhang, Yanjuan Gao, Yanhong Luo, Xiao Zhang

期刊论文

Chemical characteristics of fine particulate matter emitted from commercial cooking

Bing PEI,Hongyang CUI,Huan LIU,Naiqiang YAN

期刊论文

Particulate matter 2.5 triggers airway inflammation and bronchial hyperresponsiveness in mice by activating

期刊论文

Seasonal variations in leaf capturing of particulate matter, surface wettability and micromorphology

Huixia WANG, Hui SHI, Yangyang LI, Ya YU, Jun ZHANG

期刊论文

Particulate matter and metals partitioning in highway rainfall-runoff

Gaoxiang YING, John J. SANSALONE,

期刊论文

A method for quantifying bias in modeled concentrations and source impacts for secondary particulatematter

Cesunica E. Ivey, Heather A. Holmes, Yongtao Hu, James A. Mulholland, Armistead G. Russell

期刊论文

Concentrations of toxic heavy metals in ambient particulate matter in an industrial area of northeastern

PIAO Fengyuan, SUN Xiance, LIU Shuang, YAMAUCHI Toru

期刊论文

Long-term trends of fine particulate matter and chemical composition in the Pearl River Delta Economic

Xuemei WANG,Weihua CHEN,Duohong CHEN,Zhiyong WU,Qi Fan

期刊论文

Photoaging mechanism of microplastics: a perspective on the effect of dissolved organic matter in natural

期刊论文

Airborne bacteria associated with particulate matter from a highly urbanised metropolis: A potential

期刊论文

Determination of polyfluoroalkyl compounds in water and suspended particulate matter in the river Elbe

Lutz AHRENS, Merle PLASSMANN, Zhiyong XIE, Ralf EBINGHAUS

期刊论文

Identification of sources, characteristics and photochemical transformations of dissolved organic matter

期刊论文

Photosensitivity sources of dissolved organic matter from wastewater treatment plants and their mediation

期刊论文

Assessing the premature death due to ambient particulate matter in China’s urban areas from 2004 to 2013

Guoxia MA, Jinnan WANG, Fang YU, Xiaomin GUO, Yanshen ZHANG, Chao LI

期刊论文

Dilution sampling and analysis of particulate matter in biomass-derived syngas

Xiaoliang WANG, Curtis ROBBINS, S. Kent HOEKMAN, Judith C. CHOW, John G. WATSON, Dennis SCHUETZLE

期刊论文